I don't think android has ntfs support out of the box. I'm not positive but I do think you could accomplish getting file sizes larger than 4gig with one of the native file systems in android ext2, ext3, or ext4. however windows would not recognize the disk as its not a native windows file system.
There do seem to be a few programs in the play store that say they support ntfs but they require that the device be rooted in order to work.
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