Can you be a little more specific and tell exactly which theme you downloaded? Some themes are for some apps only, perhaps you downloaded one of those. If that is the case, it will always be mentioned in the download page.
Heres something from the Google Chrome GDE Theme download page in the market
This is a theme for the new home screen replacement- GDE.
It is based loosely on the Google Chrome theme.
***MUST HAVE GDE INSTALLED FROM THE MARKET FOR IT TO WORK****
for more info on GDE : GDE - Version 0.4.0.1 in the market! - xda-developers
So you need to have the home screen replacement GDE installed to use this theme. If you already have GDE installed, most probably you can change the theme from the app settings.
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