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I am also getting the same error trying to back up my Galaxy S3 and this is the only page on the internet I can find about this particular error shown while Kies is doing a backup:
"the following items were excluded from backup due to a system memory"
Kies warns before the backup initialises that it is not backing up Applications, of which I have 384mb of apps due to system memory on the device.
At the end of the backup, as long as I uncheck Applications - otherwise Backup fails every time - I get a list of items which could not be backed up due to the error shown above, these are:
Message, Email, Preferences and ringtones, Network settings and bookmarks, Call log, Applications, S Memo.
By device, does this mean the phone or my laptop? I have a fairly high spec laptop with 8gb RAM on Windows XP Pro x64.
What does this error mean and how can I resolve it?
Thanks for your suggestions.